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ChemicalBook CAS DataBase List 3-Ethynylpiperidine hydrochloride
959918-19-5

3-Ethynylpiperidine hydrochloride synthesis

1synthesis methods
1-Piperidinecarboxylic acid, 3-ethynyl-, 1,1-dimethylethyl ester

664362-16-7

3-Ethynylpiperidine hydrochloride

959918-19-5

General procedure for the synthesis of 3-ethynylpiperidine hydrochloride from 3-ethynylpiperidine-1-carboxylic acid tert-butyl ester: Preparation of Intermediate 35 (Method V); Synthesis of 3-ethynylpiperidine hydrochloride: to Intermediate 33 (1.50 g, 7.18 mmol) was added a dioxane solution (50 mL) of 4 M HCl. The reaction mixture was stirred at room temperature for 16 hours. After completion of the reaction, the mixture was concentrated in vacuum. The residue was ground with ether (Et2O) to give 3-alkynylpiperidine hydrochloride (0.91 g, 86% yield).1H NMR (DMSO-d6) δ: 9.02 (2H, br.s), 3.38-3.24 (1H, m), 3.21-3.08 (2H, m), 2.94-2.76 (3H, m), 2.00-1.87 (1H, m), 1.83-1.73 (1H, m), 1.73-1.60 (1H, m), 1.60-1.48 (1H, m).

664362-16-7 Synthesis
1-Piperidinecarboxylic acid, 3-ethynyl-, 1,1-dimethylethyl ester

664362-16-7
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$43.00/100mg

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Yield: 86%

Reaction Conditions:

with hydrogenchloride in 1,4-dioxane at 20; for 16 h;

Steps:


INTERMEDIATE 35 (METHOD V); 3-Ethynylpiperidine hydrochloride; To Intermediate 33 (1.50 g, 7.18 mmol) was added HCl (4iVm dioxane, 50 mL). The reaction mixture was stirred at r.t. for 16 h and concentrated in vacuo. Trituration with Et2O gave the title compound (0.91 g, 86%). δH (DMSOd6) 9.02 (2H, br. s), 3.38- 3.24 (IH, m), 3.21-3.08 (2H, m), 2.94-2.76 (3H, m), 2.00-1.87 (IH, m), 1.83-1.73 (IH, m), 1.73-1.60 (IH, m), 1.60-1.48 (IH, m).

References:

UCB PHARMA S.A. WO2007/141504, 2007, A1 Location in patent:Page/Page column 59