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57250-86-9

2-Methylamino-1,3-thiazole-4-carboxylic acid ethyl ester synthesis

2synthesis methods
-

Yield:57250-86-9 94%

Reaction Conditions:

Stage #1: formaldehydwith sodium cyanide;ammonium acetate;water at 100; for 0.5 h;Green chemistry;
Stage #2: Benzoyl isothiocyanate at 100; for 0.333333 h;Green chemistry;
Stage #3: ethyl Bromopyruvate at 100; for 1 h;Green chemistry;

Steps:

2.3. General Procedure for the Preparation of Compounds 4

General procedure: The mixture of the aldehydes 1 (2 mmol), ammoniumacetate (5 mmol), NaCN (5 mmol) and KF/CP (10 mol%) inwater (5 mL) at 100 °C stirred for 30 min. After this timebenzoyl isothiocyanate 2 (2 mmol) was added slowly. Thismixture stirred for 20 min. After that, alkyl bromides 3 (2mmol) was added. After 1 h, the reaction completed and itwas confirmed by TLC. Finally, the reaction mixture cooledto room temperature and the solid residue was collected byfiltration. The solid was washed with EtOAc and KF/CP NPsseparated. The solvent was evaporated and the product 4 wasseparated as a solid form and purified by washing with theEt2O.

References:

Hamedani, Naghmeh Faal;Azad, Leila;Shafiee, Shahin;Noushin, Annataj [Combinatorial Chemistry and High Throughput Screening,2021,vol. 24,# 1,p. 88 - 97]